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performances. 187 Two additional catalyst systems are unusual in the sense that they do not contain a transition metal. Al203/Me4Sn has been reported to bring about metathesis of propene, I-hexene, and 2-pentene. 188 Si02, in tum, shows activity in the metathesis of ethene and propene under irradiation when pretreated at high temperature under vacuum. 189 Heterogenization by attaching the Grubbs catalyst to a phosphinated mesoporous support (MCM-41) was also successful. I90 Electron-deficient (having less than 18 electrons) and coordinatively unsaturated (containing less than 6, usually only 4 or 5 ligands) metal carbene complexes are highly effective in metathesis.191-194 Particular attention has been paid to the tetracoordinated alkylidene catalysts M(=CHCMe2Ph)(=NAr)(ORh (M = Mo, W) with bulky substituents Ar and R on the imido and alkoxide ligands developed by Schrock and coworkers. 195 Similarly, ruthenium complexes Ru( =CHR)(Xh(PR' 3h (X = CI, Br, OOCCF3) developed by Grubbs and coworkers I94 ,196,197 have attracted much attention. Among them, complex 10 turned out to have high activity, but it is quite sensitive toward oxygen and moisture. Grubbs' catalysts, including the most active 11, however, generally tolerate various functional groups, are stable to air and water, and are easy to prepare and capable of inducing the metathesis of all kinds of alkenes. Some even catalyze the metathesis of 2-pentene and cycloalkenes of low strain: 192,193

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The element at the origin is denoted as + 0. -

In these equations subscripts are attached t o the mass and charge to signify that, on account of the interactions, the mass and charge parameters appearing in the Lagrangian will not generally be the physical mass and charge. This implies a process of renormalization between the bare and physical quantities that will be discussed in Chs. 3 and 6. In the interest of compact notation we will usually omit these subscripts, with the implicit understanding that physical parameters are always renormalized parameters. The equations of motion for the coupled electron and photon fields follow from independent variation of the Lagrangian density (2.202) with respect to these fields (Exercise 2.16):

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